228 results for group: journal-article

Leveraging ecosystems responses to enhanced rock weathering in mitigation scenarios

Yann Gaucher, Katsumasa Tanaka, Daniel J. A. Johansson, Daniel S. Goll, Philippe Ciais ABSTRACT: Carbon dioxide removal (CDR) is deemed necessary to attain the Paris Agreement’s climate objectives. While bioenergy with carbon capture and storage (BECCS) has generated substantial attention, sustainability concerns have led to increased examination of alternative strategies, including enhanced rock weathering (EW). We analyse the role of EW under cost-effective mitigation pathways, by including the CDR potential of basalt applications from silicate weathering (geochemical CDR) and enhanced ecosystem growth and carbon storage in response to phospho...

Bridging time lags in durable carbon removal on working lands

Noah J. Planavsky, Beck J. Woollen, Ella Milliken, Mojtaba Fakhraee, David J. Beerling, Christopher T. Reinhard ABSTRACT: Enhanced weathering and biochar application on working lands show promising signs of delivering durable carbon dioxide removal required to meet internationally agreed upon climate change mitigation goals. Although both technologies can scale comparatively quickly, their ability to offset radiative forcing from anthropogenic greenhouse gas emissions is delayed by time lags between deployment and realized carbon removal. Here, we suggest that coupling enhanced weathering and biochar with point-source methane emissions reductions ...

Atmospheric carbon dioxide mineralisation in anthropogenically-derived carbonate deposits

John MacDonald, Charlotte Slaymark, Amanda Stubbs, Marta Kalabová ABSTRACT: Removing carbon dioxide from the atmosphere is important in minimising the impact of anthropogenically-induced climate change. Anthropogenic geomaterials, such as slag and cement, can be utilised in an engineered context for mineralising CO2. However, such anthropogenic geomaterials, typically waste products, were usually deposited on the land surface and left to passively mineralise CO2, resulting in the formation of anthropogenic carbonates. In this study, we document anthropogenic carbonates from a suite of locations across Scotland and Northern England, and use stable ...

Efficient denitrification and N2O mitigation in low-C/N wastewater treatment by promoting TCA cycle anaplerosis via glyoxylate shunt regulation

Haojin Peng, Qingran Zhang, Yu Su, Shuai Wang, Yinguang Chen   ABSTRACT: Conventional biodenitrification for water with a low carbon-to-nitrogen ratio (C/N) demands exogenous carbon, exacerbating carbon consumption and emissions. Here we propose a metabolic reprogramming strategy leveraging Mo(VI)–Fe(III)–Cu(II) synergy to redirect carbon flux through the glyoxylate shunt (GS), enhancing tricarboxylic acid cycle anaplerosis for efficient denitrification and reduced greenhouse gases during low-C/N wastewater treatment. At a C/N of 3, Mo(VI)–Fe(III)–Cu(II) promoted carbon metabolism by the tricarboxylic acid cycle in Paracoccus ...

An Analysis of Soil CO₂ Efflux and Leachate Alkalinity Data

Dirk Paessler, Jens Hammes, Anna Anke Stöckel, Ralf Steffens, Ingrid Smet ABSTRACT: In order to better understand Enhanced Weathering (EW) we ran an extensive greenhouse experiment with more than 400 pots with grass plants (Lollium perenne) for 24 months throughout 2023-2024. Every month we measured multiple parameters in the soil leachate water (total alkalinity (TA), pH, electrical conductivity (EC), and cations) as well as soil CO₂ effluxes. With a focus on carbon transport we present here the data from 67 rock-soil variations with 4 replicates each, based on the lab results from 6,500 leachate samples and almost 1 million CO₂ efflux ...

Divergent responses of carbon and nitrogen functional genes composition to enhanced rock weathering

Qiong Chen, Daniel S. Goll, Mardin Abdalqadir, Xinjian He, Guochen Li, Boyuan Bi, Tongtong Xu, Chenlu Li, Yanlong Chen, Xiulian Ma, Zhenxin Li, Yunting Fang, Zhanqing Hao & Zuoqiang Yuan ABSTRACT: Enhanced rock weathering (ERW) is a scalable strategy for atmospheric carbon dioxide removal. The microbiome function critically regulates the below-ground cycle of carbon and nitrogen in terrestrial ecosystems. However, microbial functioning related to carbon and nitrogen under ERW remains elusive. Here we investigated how wollastonite addition affects key microbial carbon and nitrogen-cycles genes investigated using metagenomic, in a tropic rubber ...

Limited carbon sequestration potential from global ecosystem restoration

Csaba Tölgyesi, Nándor Csikós, Vicky M. Temperton, Elise Buisson, Fernando A. O. Silveira, Caroline E. R. Lehmann, Péter Török, Zoltán Bátori, Ákos Bede-Fazekas ABSTRACT: Ecosystem restoration is increasingly recognized as a means of climate change mitigation. Recent global-scale studies have suggested that ecosystem restoration could offset a substantial fraction of human carbon emissions since the Industrial Revolution. However, global carbon sequestration potential remains uncertain due to the tree-centric view of some models and difficulties in modelling restoration across different ecosystem types. Here we applied a model-based ...

Impact of Basalt Rock Powder on Ryegrass Growth and Nutrition on Sandy and Loamy Acid Soils

Charles Desmalles, Lionel Jordan-Meille, Javier Hernandez, Cathy L. Thomas, Sarah Dunham, Feifei Deng, Steve P. McGrath and Stephan M. Haefele ABSTRACT: Enhanced weathering of silicate rocks in agriculture is an option for atmospheric CO2 removal and fertility improvement. The objective of our work is to characterise some of the agricultural consequences of a basaltic powder amendment on soil-crop systems. Two doses of basalt (80 and 160 t ha−1) were applied to two types of slightly acid soils (sandy or silty clayey), derived from long-term trials at Bordeaux (INRAE, France) and Rothamsted Research (England), respectively. For each soil, half of ...

Increased soil CO2 emissions after basalt amendment were partly offset by biochar addition in an urban field experiment

Jennifer Newell,Rory Doherty, Gary Lyons ABSTRACT: Enhanced weathering (EW) and biochar amendment are proposed carbon dioxide removal (CDR) techniques with potential co-benefits for soil health and plant productivity. However, knowledge gaps remain regarding their impacts on soil carbon dynamics and heavy metal mobility. This study investigates the effects of basalt and biochar amendments on soil CO2 efflux (SCE), soil base cation dynamics, biomass yield and heavy metal uptake in clover (Trifolium pratense) and mustard (Brassica juncea) field plots. Despite potential CO2 uptake through weathering, we found that basalt increased SCE in both crops, ...

Pyrogenic carbon and Carbonating Minerals for Carbon Capture and Storage (PyMiCCS) Part II: Organic and Inorganic Carbon Dioxide Removal in an Oxisol

Maria-Elena Vorrath, Thorben Amann, Johannes Meyer zu Drewer, Nikolas Hagemann, Cierra Aldrich, Janine Börker, Maria Seedtke, Joscha N. Becker, Mathilde Hagens, Annette Eschenbach, Jens Hartmann ABSTRACT: Enhanced rock weathering (ERW) and pyrogenic carbon capture and storage (PyCCS, or "biochar carbon removal") are two promising carbon dioxide removal (CDR) techniques that can contribute to soil restoration. These technologies can be combined by co-application of rock powder and biochar or by co-pyrolysis of rock powder with biomass to produce rock-enhanced (RE) biochar. In a 27-week laboratory experiment, we quantified the carbon (C) sink ...